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Portrait of Alex Vermeulen

Alex Vermeulen

Manager

Portrait of Alex Vermeulen

H-2 vertical profiles in the continental boundary layer : measurements at the Cabauw tall tower in The Netherlands

Author

  • M. E. Popa
  • Alex Vermeulen
  • W. C. M. van den Bulk
  • P. A. C. Jongejan
  • A. M. Batenburg
  • W. Zahorowski
  • T. Rockmann

Summary, in English

In-situ, quasi-continuous measurements of atmospheric hydrogen (H-2) have been performed since October 2007 at the Cabauw tall tower station in the Netherlands. Mole fractions of H-2, CO and several greenhouse gases are determined simultaneously in air sampled successively at four heights, between 20 and 200 m above ground level. Rn-222 measurements are performed in air sampled at 20 and 200 m. This H-2 dataset represents the first in-situ, quasi-continuous long-term measurement series of vertical profiles of H-2 in the lower continental boundary layer. Seasonal cycles are present at all heights in both H-2 and CO, and their amplitude varies with the sampling height. The seasonality is evident in both the "baseline" values and in the short term (diurnal to synoptic time scales) variability, the latter being significantly larger during winter. The observed H-2 short term signals and vertical gradients are in many cases well correlated to other species, especially to CO. On the other hand, H-2 has at times a unique behaviour, due to its particular distribution of sources and sinks. Our estimation for the regional H-2 soil uptake flux, using the radon tracer method, is (-1.89 +/- 0.26) x10(-5) g/(m(2) h), significantly smaller than other recent results from Europe. H-2/CO ratios of the traffic emissions computed from our data, with an average of 0.54 +/- 0.07 mol: mol, are larger and more variable than estimated in some of the previous studies in Europe. This difference can be explained by a different driving regime, due to the frequent traffic jams in the influence area of Cabauw. The H-2/CO ratios of the large scale pollution events have an average of 0.36 +/- 0.05 mol:mol; these ratios were observed to slightly increase with sampling height, possibly due to a stronger influence of soil uptake at the lower sampling heights.

Publishing year

2011

Language

English

Pages

6425-6443

Publication/Series

Atmospheric Chemistry and Physics

Volume

11

Issue

13

Document type

Journal article

Publisher

Copernicus GmbH

Topic

  • Physical Geography

Status

Published

ISBN/ISSN/Other

  • ISSN: 1680-7324