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No particle mass enhancement from induced atmospheric ageing at a rural site in northern Europe

Författare:
  • Erik Ahlberg
  • Stina Ausmeel
  • Axel Eriksson
  • Thomas Holst
  • Tomas Karlsson
  • William H. Brune
  • Göran Frank
  • Pontus Roldin
  • Adam Kristensson
  • Birgitta Svenningsson
Publiceringsår: 2019-07-17
Språk: Engelska
Publikation/Tidskrift/Serie: Atmosphere
Volym: 10
Nummer: 7
Dokumenttyp: Artikel i tidskrift
Förlag: MDPI AG

Abstract english

A large portion of atmospheric aerosol particles consists of secondary material produced by oxidation reactions. The relative importance of secondary organic aerosol (SOA) can increase with improved emission regulations. A relatively simple way to study potential particle formation in the atmosphere is by using oxidation flow reactors (OFRs) which simulate atmospheric ageing. Here we report on the first ambient OFR ageing experiment in Europe, coupled with scanning mobility particle sizer (SMPS), aerosol mass spectrometer (AMS) and proton transfer reaction (PTR)-MS measurements. We found that the simulated ageing did not produce any measurable increases in particle mass or number concentrations during the two months of the campaign due to low concentrations of precursors. Losses in the reactor increased with hydroxyl radical (OH) exposure and with increasing difference between ambient and reactor temperatures, indicating fragmentation and evaporation of semivolatile material.

Keywords

  • Meteorology and Atmospheric Sciences
  • Ambient aerosol
  • Oxidation flow reactor
  • PAM
  • Secondary organic aerosol

Other

Published
  • ISSN: 2073-4433
E-post: tomas [dot] karlsson [at] nateko [dot] lu [dot] se

Doktorand

Institutionen för naturgeografi och ekosystemvetenskap

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Institutionen för naturgeografi och ekosystemvetenskap
Lunds universitet
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223 62 Lund
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